Energetic aluminum cluster deposition has been investigated with a classica
l molecular dynamics simulation and the Metropolis Monte Carlo simulation u
tilizing the second-moment approximation of the tight-binding scheme, when
a local area became a melting state on the surface around the impact point
of an energetic aluminum cluster during a few ps, intermixing easily occurr
ed and a good epitaxial film with bulk density was formed. For excellent fi
lm growth using cluster impact, it is necessary to make the local area temp
erature higher than the melting temperature on the surface around the impac
t point of an energetic cluster.