S. Lettieri et al., Measurements of the nonlinear refractive index of freestanding porous silicon layers at different wavelengths, PHIL MAG B, 81(2), 2001, pp. 133-139
Measurements of the nonlinear refractive index n(2) of a high-porosity free
standing porous silicon sample are reported at different laser wavelengths
by means of the z-scan technique. The results show a negative below-gap non
linear refractive index, so that thermal contributions to the observed effe
cts can be reasonably excluded. Values for n(2) of the order of 10(-9) esu
are here reported. These results are compatible with the hypothesis of an e
nhancement of optical nonlinearities due to quantum confinement of carriers
in nanocrystals present in the material.