This paper presents a study of BaFe12-2xTixCoxO19, where the substitution-i
nduced magnetic anisotropy change has been investigated through magnetic me
asurements and single-crystal neutron diffraction. The study shows that the
magnetic structures of BaFe12-2xTxCoxO19 change drastically when the tempe
rature and the substitution rate are altered. It is proposed that an antife
rromagnetic mode in doped Ba-hexaferrites is one of the key elements to und
erstand the origin of their promising microwave properties. (C) 2001 Elsevi
er Science B.V. All rights reserved.