The thermal conductivity of both LEO and HVPE single crystals of GaN have b
een measured over the temperature range of 60 K to 300 K using an electrica
l third harmonic technique. In contrast to the previously reported results
of Sichel and Pankove, the thermal conductivity increases with decreasing t
emperature below room temperature, reaches a maximum and then decreases wit
h further decreases in temperature. The thermal conductivity of the LEO-GaN
is higher at all temperatures than the HVPE materials. The higher thermal
conductivity is correlated with lower values of the threading dislocation d
ensity.