The monthly-mean total chlorine abundance (CL) at 55 km inferred from HALOE
HCl observations increases from 1992 to 1997 and then subsequently decreas
es. The pre-1997 increase is consistent with surface measurements of Cl-T t
ime-lagged by around 6 years. However, a decrease after 1997 is inconsisten
t with such a time lag, which would predict a peak in late 1999. Accounting
for stratospheric mixing processes produces an expected stratosphere CIT w
hich is in agreement with the HALOE Cl-T time series considering the uncert
ainty in the HALOE data. However, the peak in Cl-T is still predicted to oc
cur in later 1999 rather than 1997. We find that reasonable low frequency c
hanges in transport, chlorine partitioning, anomalous buildup of organic ch
lorine at 55 km, and tropospheric rainout of inorganic chlorine do not reco
ncile the expected and HALOE Cl-T time series. At present, we are unable to
explain hear upper stratospheric Cl-T could decrease as early as 1997.