Nonlinear electron current through a short molecular wire

Citation
Eg. Petrov et P. Hanggi, Nonlinear electron current through a short molecular wire, PHYS REV L, 86(13), 2001, pp. 2862-2865
Citations number
21
Categorie Soggetti
Physics
Journal title
PHYSICAL REVIEW LETTERS
ISSN journal
00319007 → ACNP
Volume
86
Issue
13
Year of publication
2001
Pages
2862 - 2865
Database
ISI
SICI code
0031-9007(20010326)86:13<2862:NECTAS>2.0.ZU;2-R
Abstract
The voltage and the temperature behavior of inelastic interelectrode curren t mediated by a short molecular wire is analyzed within a nonlinear kinetic approach that accounts for strong Coulomb repulsion between transferring e lectrons. When the coupling to the heat bath occurs via high-frequency vibr ation modes we predict a generally nonlinear current-voltage characteristic s (an Ohmic behavior at small voltage, rising towards saturation and being followed by an abrupt decrease at large voltage) and a bell-shaped current response vs temperature at not too large temperatures.