A finite-mode probability density function method was used with a computati
onal fluid dynamics cone to model the semibatch precipitation of barium sul
fate from aqueous solutions of barium chloride and sodium sulfate in a Tayl
or-Couette reactor: It was simulated in turbulent flow at high Taylor numbe
rs under the assumption of axial symmetry. The flow field was modeled using
two different turbulence model and flow predictions were validated using e
xperimental tracer dispersion measurements. The crystal-size distribution (
CSD) was calculated in terms of the first five moments considering both nuc
leation and growth, while neglecting the effect of aggregation. The effect
of the operating conditions on the CSD was studied, and code predictions we
re compared with experimental data.