We reexamine the possibility of resolving 3D density structure in the mantl
e, by performing test inversions using a dataset of well constrained degree
2 splitting coefficients. We show that degree 2 in V-s and V-p can be reso
lved, and confirm that dlnV(s)/dlnV(p) >2.5 at depths > 2000km, indicating
a chemical component to large scale heterogeneity. Models with rho positive
ly correlated with V-s in the deepest mantle fit the data at least as well
as those in which density and velocities are anti-correlated. However, some
rough bounds on dln rho /dlnV(s) can be inferred. Models obtained from geo
dynamic considerations are acceptable, in contrast to models with large neg
ative (< -0.3) or positive (> 0.6) dln rho /dlnV(s) throughout the lower ma
ntle. The most robust feature is a marked increase in dln rho /dlnV(s) at t
he top of the lower mantle reaching a maximum around 1500 km.