Universality of the Stokes shift for a disordered ensemble of quantum dots

Citation
A. Patane et al., Universality of the Stokes shift for a disordered ensemble of quantum dots, PHYS ST S-B, 224(1), 2001, pp. 41-45
Citations number
10
Categorie Soggetti
Apllied Physucs/Condensed Matter/Materiales Science
Journal title
PHYSICA STATUS SOLIDI B-BASIC RESEARCH
ISSN journal
03701972 → ACNP
Volume
224
Issue
1
Year of publication
2001
Pages
41 - 45
Database
ISI
SICI code
0370-1972(200103)224:1<41:UOTSSF>2.0.ZU;2-5
Abstract
We present a study of carrier redistribution in InxGa1-xAs/GaAs self-assemb led quantum dots (QDs) by comparing electroluminescence (EL) and photocurre nt (PC) spectra. We show the: existence of a red-shift of the dot emission in EL relative to the dot absorption in PC, referred to as the Stokes shift (SS). The existence of the SS is explained in terms of a thermal redistrib ution of carriers between dots. According to the thermalization model, the SS increases with the linewidth of the QD absorption spectrum. We show that for a large variety of quantum dots, differing in the material system and/ or the growth technique, the SS has a universal dependence on the QD absorp tion linewidth.