Transverse and in-plane modification of superconductivity and electronic structure in the quasi-two-dimensional organic conductor kappa-(BEDT-TTF)(2)Cu(SCN)(2) by uniaxial stress

We have employed uniaxial stress along the principal axes of the quasi-two- dimensional organic superconductor kappa-(BEDT-TTF)(2)Cu(SCN)(2) (BEDT-TTF = bis(ethylenedithio)tetrathiafulvalene). The lattice anisotropy is there b y altered, with corresponding changes in the intermolecular transfer energi es. The effect of uniaxial stress on the superconducting transition tempera ture T-c and critical field B-c2 is found to be anisotropic. There is an in dication of an increase in T-c and an increase in B-c2 for in-plane stress, but both parameters decrease rapidly for transverse (interplane) stress. M agnetotransport studies reveal stress-induced changes in the Fermi surface through the observation of the Shubnikov-de Haas oscillations. The stress d ependence of a resistive anomaly in the magnetoresistance, which is associa ted with the critical field B-c2 is also investigated. We discuss the exper imental findings in the context of recent phenomenological and theoretical treatments of quasi-two-dimensional systems where the anisotropic triangula r-lattice Hubbard model has been used to treat two-dimensional superconduct ors.