The phenomenon of radial plutonium migration in fast reactor MOX fuel is on
e of the important performance issues. In this study, mechanisms of this ph
enomenon were modeled for vapor transport concurrently occurring with therm
al diffusion. Further improvement was modeled by accounting for the effects
of the oxygen to metal ratio. Additionally, to evaluate more precisely the
fuel temperature history during irradiation, the thermal conductivity in t
he fuel-cladding gap was evaluated by including the thermal effects of fiss
ion-product (FP) compounds. The calculated plutonium distribution in MOX fu
el irradiation tests, with the linear heat rate (LHR) gradually decreasing
with irradiation, agreed well with the measured data. improvement by consid
ering the effect of the oxygen to metal ratio was considered to be effectiv
e and indispensable for the evaluation of plutonium migration in the MOX fu
el. (C) 2001 Elsevier Science B.V. All rights reserved.