Magnetic ultrathin alloy films CoxNi1-x/Cu(100) were prepared to characteri
ze the behavior of spin reorientation transition (SRT). With the double cal
ibration by medium energy electron diffraction oscillation and Auger electr
on spectroscopy, the composition of the alloy films was controlled within a
n accuracy of +/-0.5%. which allowed us to prepare alloy films in very low
Co concentration. The critical thickness of SRT in alloy ultrathin films Co
xNi1-x/ Cu(100) was significantly delayed for x less than 10%. and for x =
10% alloy films, at least up to 20.6 ML, always revealed in-plane anisotrop
y. Besides the sensitive influence of composition on SRT behavior when x le
ss than or equal to 10%, the vertical interlayer distance of all the films
did not show any significant difference. These results were consistent with
prior theoretical calculation, in which the magnetic anisotropy was conclu
ded to change sign abruptly while tuning a few average number of 3d electro
n. (C) 2001 Published by Elsevier Science B.V.