New models of Mercury's internal structure are calculated for different amo
unts of sulfur in the core. The density of an FeS core differs by only abou
t 0.5% from the mean density of Mercury. A determination of Mercury's momen
t of inertia will effectively discriminate among the models and place relat
ively tight constraints on the radius and sulfur content of the core despit
e relatively large uncertainties in the density and temperature of the sili
cate mantle. (C) 2001 Academic Press.