Using computer-controlled pulsed laser deposition, high quality SrMoO3 thin
films have been epitaxially grown on SrTiO3 (001) substrates. A growth int
erruption technique was employed for better epitaxy, and layer-by-layer gro
wth was obtained by the intensity oscillations of reflection high-energy el
ectron diffraction. The films were of epitaxial crystallinity as characteri
zed by high-resolution transmission electron microscopy. The typical root m
ean square surface roughness was 2.2 Angstrom. The SrMoO3 thin films showed
metal-like conducting behavior with resistivity on the order of 60-120 mu
Omega cm between 4 K and room temperature. An x-ray photoelectron spectrosc
opy study shows that the valence band spectrum of the film has the typical
character of a metal, and Mo 4dt(2g) electrons an responsible fur the condu
ction of the films. (C) 2001 American Vacuum Society.