We review our recent proposal for a unified, microscopic, many-body theory
for the 2:1 organic charge transfer solids (CTS), which range from nearly 1
D to strongly 2D in electronic character. Our theory predicts an insulating
bond-charge density wave (BCDW) ground state in the limit of exact 1/4-fil
ling for all anisotropies, consistent with experimental observations of coe
xisting density waves in the real materials. For weakly 2D materials, we fi
nd that a spin-density wave (SDW) coexists with the BCDW; the resulting BCS
DW is again consistent with experiments. In contrast, both in the 1D limit
and in the strongly 2D regime the systems can be in the nonmagnetic singlet
state. We suggest that slightly away from exact 1/4-filling, commensurabil
ity defects can form pairs leading to superconductivity.