T. Hasegawa et al., Donor-acceptor-type complexes of (BEDT-TTF)(TCNQ) analogues: Peculiar magnetic transition in (BEDO-TTF)(Cl(2)TCNQ), SYNTH METAL, 120(1-3), 2001, pp. 991-992
This report presents electronic properties of an ionic mixed-stack charge-t
ransfer compound, (BEDO-TTF)(Cl(2)TCNQ), which is a magnetic insulator exhi
biting Curie-Weiss behavior in magnetic susceptibility followed by a sharp
drop at around 100 similar to 120K. The vibronic spectra of this compound a
t low temperature clearly indicate that the observed magnetic anomaly is Pl
ot associated with the conventional "spin-Peierls"-like dimeric lattice dis
tortions.