Me. Chang et al., ON USING INVERSE METHODS FOR RESOLVING EMISSIONS WITH LARGE SPATIAL INHOMOGENEITIES, JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 102(D13), 1997, pp. 16023-16036
We apply an inverse method to estimate the carbon monoxide emissions i
n Atlanta, Georgia. The resultant carbon monoxide inventory is unreali
stically characterized by temporal oscillations on the frequency of 1
hour. We suspect that the difficulty in deducing the emissions is due
to inhomogeneities in the spatial distribution of the emissions. In se
veral controlled experiments we reproduce the oscillations by introduc
ing relatively small errors into the spatial distribution of the emiss
ion inventory. In similar experiments with isoprene in which the emiss
ions are more homogeneous, we do not find this problem. These results
are discussed in the context of previous inverse studies of carbon mon
oxide and isoprene.