The exchange interactions in polycrystalline samples of Ca1-xLaxMnO3 (0.00
less than or equal to x less than or equal to 0.05) are studied by means of
Raman scattering and electron paramagnetic resonance. Dramatic reductions
in the spin-phonon interactions and magnetic correlations are observed for
La doping levels as small as similar to2%-3%. These results show that the c
harge carriers play an important role in the overall exchange coupling in t
he electron-doped manganites, even at very low doping levels.