The physics of soft materials can be investigated using nuclear spin-lattic
e relaxation, which depends on the spectral densities of motion in the MHz
range. For the first time, NMR relaxation has been used to study influences
of the acyl length, polar head groups, a cosurfactant, and cholesterol on
the viscoelastic properties of membrane lipids. The results imply the conce
pt of elastic deformation is relevant on lengths approximate to the bilayer
thickness and less, involving a broad spectrum of collective modes which c
ontribute to the forces between lipid bilayers.