Advective coalescence in chaotic flows - art. no. 038301

We investigate the reaction kinetics of small spherical particles with iner tia, obeying coalescence type of reaction, B + B --> B, and being advected by hydrodynamical flows with time-periodic forcing. In contrast to passive tracers, the particle dynamics is governed by the strongly nonlinear Maxey- Riley equations, which typically create chaos in the spatial component of t he particle dynamics, appearing as filamental structures in the distributio n of the reactants. Defining a stochastic description supported on the natu ral measure of the attractor, we show that, in the Limit of slow reaction, the reaction kinetics assumes a universal behavior exhibiting a t(-1) decay in the amount of reagents, which become distributed on a subset of dimensi on D-2, where D-2 is the correlation dimension of the chaotic flow.