New methods of generation of anti-Stokes radiation of stimulated Raman scat
tering in media with changeable parameters of the third-order nonlinearity
chi ((3)) along the longitudinal coordinate are proposed. The conditions of
obtaining phase quasi-matching in different media and reaching the maximum
efficiency of conversion into the anti-Stokes component of stimulated scat
tering are determined by numerical methods. The dependence of the efficienc
y of energy transfer from the pump wave to the anti-Stokes wave on the rati
o of intensities of the pump and Stokes waves at the input of the medium is
studied. The models of the media in which the efficiency of generation of
anti-Stokes radiation exceeds 30% are obtained. The results of the investig
ation can be used for the development of new efficient nonlinear optical de
vices upconverting the laser radiation frequency. (C) 2001 MAIK "Nauka/Inte
rperiodica".