Thin FePt (001) films, grown by molecular-beam epitaxy on Pt(001), exhibit
a very large perpendicular magnetic anisotropy (K-u=5x10(6) J m(-3)) and a
100% magnetic remanence in perpendicular field. The lattice misfit between
FePt and Pt (1.5%) relaxes through the pileup of a/6 < 112 > partial disloc
ations along {111} planes, leading to the formation of microtwins. Atomic f
orce microscopy images demonstrate that this process induces a spontaneous
rectangular nanostructuration of the sample, while magnetic force microscop
y shows that the microtwins act as pinning sites for the magnetic walls. Th
is leads to square magnetic domains and explains the large coercivity assoc
iated with the domain wall propagation. (C) 2001 American Institute of Phys
ics.