Polymer-layered silicate (PLS) nanocomposites exhibit some mechanical prope
rties that are much better than conventional polymer filled composites. A r
elatively low content of layered silicate yields a significant enhancement
of material performance. After the volume fraction of clay reaches a relati
vely low "critical value"; however, further increasing does not show a grea
ter stiffening effect. This phenomenon is contrary to previous micromechani
cal predictions and Is not understood well. Based on the analysis on the mi
crostructures of PLS nanocomposites, the present note provides an insight i
nto the physical micromechanisms of the above unexpected phenomenon. The Mo
ri-Tanaka scheme and a numerical method are employed to estimate the effect
ive elastic moduli of such a composite.