Polymeric "smart" coatings have been developed that are capable of both det
ecting and removing hazardous nuclear and heavy metal contaminants from con
taminated surfaces. These coatings consist of strippable polymeric composit
ions containing blends of polymers, copolymers and additives that can be br
ushed or sprayed onto a surface as a solution or dispersion in aqueous medi
a. Upon drying, these coatings form strong films that can easily be peeled
or stripped from the surface. When applied to a contaminated surface, these
coatings display responsive behavior. Areas of contamination are indicated
by a color change. As the coatings dry, the contaminants are drawn into an
d fixed in the polymer matrix. Subsequent removal of the coating with entra
pped contaminants results in some degree of surface decontamination. Here w
e report the development and investigation of a smart, decontaminating coat
ing developed for uranium and plutonium.