Electroluminescence (EL) from silicon nanocrystals in Si/CaF2 superlattices
grown by molecular-beam epitaxy at room temperature was investigated and c
ompared with that obtained from silicon nanocrystals in Si/SiO2 superlattic
es. EL spectra exhibited current-tunability, similar to that observed in si
licon nanocrystals in SiO2, which was attributed to three main effects: (a)
Auger quenching of photoluminescence, which occurs when more than one elec
tron-hole pair is present in the same nanocrystal and which quenches lumine
scence from relatively larger nanocrystals, (b) size-dependent carrier inje
ction, and (c) the effect of the applied field, when this one is significan
tly high. In the case of Si/CaF2 superlattices, this last factor did not ap
ply, so the two other factors are mainly at the origin of the effect. (C) 2
001 American Institute of Physics.