Investigations of magnetic dilution in Y3Fe5O12 (YIG) indicate that magneti
c and dielectric parameters suitable for microwave applications can be obta
ined at cryogenic temperatures. For simultaneous dilutions of 35% into the
octahedral (a) sublattice and 27% into the tetrahedral (d) sublattice, ther
e were no apparent degrading effects on the dielectric loss tangents. At lo
w temperatures, a-site substitutions of In caused the expected large increa
ses in saturation magnetization and corresponding decreases in Curie temper
atures. Moreover, measurements of hysteresis loops showed that coercive fie
lds similar to0.5 Oe could be obtained at T < 77 K despite the likely sharp
rise in anisotropy. Dilution by In also lowered anisotropy fields by a fac
tor greater than five from that Of Y-3(Fe,AI)(5)O-12 in both {Y,Ca}(3)(Fe,V
In)(5)O-12 and Y-3(Fe,Al,In)(5)O-12 compounds.