Control, with a rf field, of photon emission times by a single molecule and its connection to laser-induced localization of an electron in a double well

Citation
De. Makarov et H. Metiu, Control, with a rf field, of photon emission times by a single molecule and its connection to laser-induced localization of an electron in a double well, J CHEM PHYS, 115(13), 2001, pp. 5989-5993
Citations number
23
Categorie Soggetti
Physical Chemistry/Chemical Physics
Journal title
JOURNAL OF CHEMICAL PHYSICS
ISSN journal
00219606 → ACNP
Volume
115
Issue
13
Year of publication
2001
Pages
5989 - 5993
Database
ISI
SICI code
0021-9606(20011001)115:13<5989:CWARFO>2.0.ZU;2-A
Abstract
We simulate an experiment in which a single molecule is simultaneously expo sed to light resonating with a transition and to rf radiation. We show how the rf radiation can be used to control the statistical properties of the p hoton emission events (e.g., the time between successive photon emissions). This process is isomorphic with laser-induced localization of an electron in a semiconductor double well. (C) 2001 American Institute of Physics.