Control, with a rf field, of photon emission times by a single molecule and its connection to laser-induced localization of an electron in a double well
De. Makarov et H. Metiu, Control, with a rf field, of photon emission times by a single molecule and its connection to laser-induced localization of an electron in a double well, J CHEM PHYS, 115(13), 2001, pp. 5989-5993
We simulate an experiment in which a single molecule is simultaneously expo
sed to light resonating with a transition and to rf radiation. We show how
the rf radiation can be used to control the statistical properties of the p
hoton emission events (e.g., the time between successive photon emissions).
This process is isomorphic with laser-induced localization of an electron
in a semiconductor double well. (C) 2001 American Institute of Physics.