High-power femtosecond laser pulses have been used to excite surface plasmo
ns in 500 Angstrom silver and gold films. Nonlinear excitation results in t
he emission of electron bunches through multiphoton excitation at low power
and laser-induced field emission at high power. The energies of photoelect
rons are found to extend as high as 0.4 keV. Calculations show that these h
igh energies are due to ponderomotive acceleration in an evanescent field e
xtending from the metal film out into the vacuum. The theoretical calculati
ons suggest that femtosecond electron pulses with relativistic energies can
be generated using longer wavelengths or by developing the surface morphol
ogy. (C) 2001 American Institute of Physics.