Carbon monoxide yield in natural gas autothermal reforming process

Authors
Citation
Sh. Chan et Hm. Wang, Carbon monoxide yield in natural gas autothermal reforming process, J POWER SOU, 101(2), 2001, pp. 188-195
Citations number
15
Categorie Soggetti
Physical Chemistry/Chemical Physics","Environmental Engineering & Energy
Journal title
JOURNAL OF POWER SOURCES
ISSN journal
03787753 → ACNP
Volume
101
Issue
2
Year of publication
2001
Pages
188 - 195
Database
ISI
SICI code
0378-7753(20011015)101:2<188:CMYING>2.0.ZU;2-Y
Abstract
This study presents the effect of natural gas (NG), composition on carbon m onoxide (CO) yield in the products of an autothermal reforming (ATR) proces s. Since NG is a mixture without definite composition, a computer routine i s coded, which is able to randomly generate various compositions whose indi vidual constituents fall within the defined ranges Then each NG is analyzed based on the AIR process within optimal ranges of the air-to-fuel ratio (A FR) and water-to-fuel ratio (WFR), which were obtained from a typical compo sition of NG under the constraints of maximum hydrogen production, minimum carbon monoxide yield, and free from solid carbon in the reformate. Finally , the correlation between NG composition and carbon monoxide yield is estab lished. This provides valuable information for the development of methods f or the clean-up of carbon monoxide. (C) 2001 Elsevier Science B.V. All righ ts reserved.