Aided by advances in modelling tools and computational power, one is now ab
le to numerically investigate grain and sub-grain heterogeneities in polycr
ystalline aggregates containing enough grains to form a representative samp
le of the relevant orientation distribution functions. Materials with multi
ple ductile phases, especially those with phases having large strength diff
erences or with strongly anisotropic single-crystal constitutive responses,
tend to undergo deformations with greater heterogeneity at the scale of gr
ains and are good candidates for numerical study. Interest in model predict
ions of grain and sub-grain deformation heterogeneities, and thus lattice o
rientation variations, has been fuelled by the automation of experimental t
echniques, such as electron back-scatter diffraction scanning. These techni
ques make it possible to obtain a rich characterization of the spatial arra
ngement of lattice orientations in a sample. Simulation results include pre
dictions of grain and sub-grain deformation heterogeneities, and emphasis i
s placed on quantities which may be compared to experimentally measured val
ues. Results for the deformation of titanium in the two-phase regime show a
relationship between spatial correlations of the misorientation structure
and both crystallographic and sample directions.