Spectral properties and infrared absorption in manganites - art. no. 144302

Within a recently proposed variational approach it has been shown that, in La(1-x)A(x)MnO(3) perovskites with 0<x<0.5, near the metal-insulator transi tion, the combined effect of the magnetic and electron-phonon interactions pushes the system toward a regime of two coexisting phases: a low electron density one made by itinerant large polarons forming ferromagnetic domains and a high electron density one made by localized small polarons giving ris e to paramagnetic or antiferromagnetic domains depending on temperature, Em ploying the above-mentioned variational scheme, in this paper spectral and optical properties of manganites are derived for x=0.3 at different tempera tures. It is found that the phase separation regime induces a robust pseudo gap in the excitation spectrum of the system. Then the conductivity spectra are characterized by a transfer of spectral weight from high to low energi es, as the temperature T decreases. In the metallic ferromagnetic phase, at low T two types of infrared absorption come out: a Drude term and a broad absorption hand due respectively to the coherent and incoherent motion of l arge polarons. The obtained results turn out in good agreement with experim ents.