P. Doussineau et al., Aging and other related phenomena in potassium niobo-tantalate crystals studied through the frequency dependence of their dielectric constant, J PHYS-COND, 13(39), 2001, pp. 8799-8816
We report on dielectric measurements in the frequency range from 1 to 1000
kHz in two disordered ferroelectric KTa1-yNbyO3 (KTN) crystals (y congruent
to 0.02). We have studied the frequency dependence of the dielectric const
ant (real and imaginary parts) during several thermal evolutions: isotherma
l aging, rejuvenation by cooling or heating after a temperature plateau, me
mory. In every case the frequency dependence is well described by a power l
aw. The temperature and plateau duration dependences of the exponents have
been studied. We give a description of our results within a model where the
variations of the dielectric constant are attributed to the motion (growth
and reconformation ) of ferroelectric domain walls. In particular we are a
ble to explain the identity of the exponents of the frequency power law dep
endence of memory and isothermal aging.