Pressure effects on the stability of magnetic phases in La1.4Sr1.6Mn2O7 hav
e been studied using magnetization measurements and neutron diffraction. At
ambient conditions this material is a quasi-two-dimensional ferromagnet. O
n cooling it becomes ordered three dimensionally: at 90 K La1.4Sr1.6Mn2O7 i
t becomes an antiferromagnet, and at 65 K it undergoes a transition into a
ferromagnetic phase. Using neutron diffraction techniques on a single cryst
al of La1.4Sr1.6Mn2O7 it has been shown that these two magnetic phases belo
ng to a single structural phase and do not coexist at low temperatures. The
application of pressure enhances the antiferromagnetic correlations betwee
n the Mn2O9 bilayers.