The CH4/NO/O-2 "lean-deNO(x)" reaction on mesoporous Mn-based mixed oxides

Authors
Stathopoulos, VN Costa, CN Pomonis, PJ Efstathiou, AM
Citation
Vn. Stathopoulos et al., The CH4/NO/O-2 "lean-deNO(x)" reaction on mesoporous Mn-based mixed oxides, TOP CATAL, 16(1-4), 2001, pp. 231-235
Citations number
23
Categorie Soggetti
Physical Chemistry/Chemical Physics
Journal title
TOPICS IN CATALYSIS
ISSN journal
10225528 → ACNP
Volume
16
Issue
1-4
Year of publication
2001
Pages
231 - 235
Database
ISI
SICI code
1022-5528(2001)16:1-4<231:TC"ROM>2.0.ZU;2-H
Abstract
High surface area Mn-based porous oxides (MANPO) containing additives like Ce, Sr and La were found to be very active and selective materials under 0. 67% CH4/0.2% NO/5% O-2 "lean-deNO(x)" conditions in the 200-300 degreesC lo w-temperature range. These materials perform also impressively in the prese nce of 4% H2O in the feed stream, where a N-2 selectivity of 98% and an exc ellent stability over 24 h on stream have been observed. The MANPO material s can be considered serious competitors of noble metals for low-temperature "lean-deNO(x) applications.