The structural and magnetic characterization of Lu2Fe17Hx (x=0; 3) single c
rystals is presented. The host alloy crystallizes with a disordered variant
of hexagonal (Th2Ni17-type P6(3)/mmc) structure, It is observed that the h
ost alloy symmetry is retained upon hydrogenation. Hydrogen is found to be
accommodated in the rare earth-rich octahedral position. The Neel temperatu
re of the hydride Lu2Fe17H3 is increased by 35 K per hydrogen atom. The mag
netization and magnetic anisotropy constant remains practically unaffected
in the hydride Lu2Fe17Hx at x=3. (C) 2001 Elsevier Science B.V. All rights
reserved.