The effects of substitution of Ru for Mn in the layered charge ordered mang
anites, La0.5Sr1.5MnO4 and LaSr2Mn2O4 have been studied by X-ray diffractio
n, magnetization and resistivity measurement techniques. The solubility of
Ru in both La0.5Sr1.5MnO4 and LaSr2Mn2O7 is much lower than that observed f
or perovskite manganites. For both the charge ordered parent compounds, the
substitution of Ru destroys charge ordering (CO), induces ferromagnetic mo
ments and improves the magneto-resistive properties. The possible origins o
f these effects are discussed. (C) 2001 Elsevier Science Ltd. All rights re
served.