Positive muons can be implanted into organic and molecular magnets in order
to study their internal magnetic field distribution and any associated dyn
amics. The muon behaves essentially as a "microscopic magnetometer", sensit
ive to local magnetic order and magnetic fluctuations. We describe some rec
ent experiments using this technique which were performed on a variety of o
rganic systems, including nitronyl nitroxide magnets and materials with spi
n-Peierls ground states, MF-M(TCNQ)(2) and DEM(TCNQ)(2), and demonstrate ho
w the technique can give information concerning their ground states.