Linear magneto-optical Kerr effect (MOKE) microscopy and magnetization-indu
ced second-harmonic-generation (MSHG) magnetometry and imaging were used as
two complementary optical techniques to measure the magnetic hysteresis lo
ops and to visualize the domain structure in Pt/Co/Pt thin films with a wea
k uniaxial in-plane magnetic anisotropy. While the MOKE is used to probe th
e magnetization over the full thickness of the Co layer, MSHG is used to ch
eck the Co/Pt interfaces selectively. When the magnetic field H is not appl
ied along the easy axis a, longitudinal MOKE and MSHG hysteresis loops exhi
bit different shapes. The differences between the longitudinal MOKE and MSH
G magnetic pattern images for H parallel to a are only found in domain wall
regions. All of these results are interpreted by considering transverse co
mponents of the non-linear optical polarization.