Sub-angstrom resolution of atomistic structures below 0.8 angstrom

Citation
Ma. O'Keefe et al., Sub-angstrom resolution of atomistic structures below 0.8 angstrom, PHIL MAG B, 81(11), 2001, pp. 1861-1878
Citations number
25
Categorie Soggetti
Apllied Physucs/Condensed Matter/Materiales Science
Journal title
PHILOSOPHICAL MAGAZINE B-PHYSICS OF CONDENSED MATTER STATISTICAL MECHANICSELECTRONIC OPTICAL AND MAGNETIC PROPERTIES
ISSN journal
13642812 → ACNP
Volume
81
Issue
11
Year of publication
2001
Pages
1861 - 1878
Database
ISI
SICI code
1364-2812(200111)81:11<1861:SROASB>2.0.ZU;2-B
Abstract
Microcharacterization of defects is greatly facilitated with improvement in resolution. By improving temporal coherence (chromatic aberration) and com pensating spatial incoherence, we have achieved the goal of the 1 Angstrom microscope (O AngstromM) project at the US Department of Energy's National Center for Electron Microscopy by extending the limits of high-resolution t ransmission electron microscopy to sub-angstrom levels. The O AngstromM com bines focal-series image-processing software with a modified 300 keV electr on microscope equipped with a highly coherent field emission electron gun. By operating at an 'alpha -null' value of underfocus in order to minimize t he effects of spatial incoherence, and by reducing the O AngstromM's electr on-gun extraction voltage to improve temporal coherence, we are able to tra nsfer information below 0.8 Angstrom In a test specimen of silicon viewed i n the [112] orientation in the O AngstromM we are able to 'see' atoms separ ated by only 0.78 Angstrom. Sub-angstrom resolution at this level offers th e materials researcher an effective tool for the characterization of defect s with unprecedented precision.