Aperiodic materials, such as two-dimensional quasicrystalline structures, s
how characteristic elements in transmission electron microscopy images that
are closely related to structure elements in the corresponding material. A
lthough the arrangement of these structure elements fundamentally influence
s the properties of the two-dimensional quasicrystalline structures, it can
not be determined in a satisfactory way by conventional diffraction-based m
ethods. We have developed an automated procedure for analysing images obtai
ned by high-resolution transmission electron microscopy. The method, which
is based on image processing, determines the two-dimensional arrangement of
the characteristic features and enables subsequent statistical data analys
is. It is illustrated with new tiling analyses of highly perfect decagonal
Al-Co-Ni quasicrystals.