Do Mie plasmons have a longer lifetime on resonance than off resonance?

Citation
M. Scharte et al., Do Mie plasmons have a longer lifetime on resonance than off resonance?, APP PHYS B, 73(4), 2001, pp. 305-310
Citations number
22
Categorie Soggetti
Apllied Physucs/Condensed Matter/Materiales Science
Journal title
APPLIED PHYSICS B-LASERS AND OPTICS
ISSN journal
09462171 → ACNP
Volume
73
Issue
4
Year of publication
2001
Pages
305 - 310
Database
ISI
SICI code
0946-2171(200109)73:4<305:DMPHAL>2.0.ZU;2-O
Abstract
The dynamics of laser-excited electrons in elliptically shaped silver nano- particles is studied using time-resolved two-photon photo-emission. By chan ging the polarization of the laser pulse at a fixed frequency, a different dynamics is observed near and far from resonance. To analyze these data , t he effect of radiation damping on Mie plasmons of Ag nanoparticles is studi ed as a function of laser frequency and polarization. It is shown that the off-resonance lifetime can be shorter or longer than the lifetime at resona nce, depending on the incidence conditions of the laser light and on the de polarization factors characterizing the optical response of the nano-partic les.