We report here new results that further elucidate the role of buoyancy-driv
en convective flows in determining the distribution of vapor mole fraction
and temperature in the thermal diffusion cloud chamber. A two-dimensional m
odel describing both diffusion and convection in the presence of chamber si
dewalls is presented. The model equations are used to analyze 1-butanol and
I-pentanol nucleation data obtained earlier. The results of the investigat
ion show that convective flow is nearly always present and, in the cases co
nsidered here, result in a reduction in the value of the calculated critica
l supersaturation (as compared to the one-dimensional case). The dependence
of critical supersaturation with total pressure reported earlier is smalle
r but is not eliminated.