The impact of convective flow on thermal diffusion cloud chamber operation

Citation
F. Ferguson et Rh. Heist, The impact of convective flow on thermal diffusion cloud chamber operation, J PHYS CH B, 105(47), 2001, pp. 11828-11833
Citations number
32
Categorie Soggetti
Physical Chemistry/Chemical Physics
Journal title
JOURNAL OF PHYSICAL CHEMISTRY B
ISSN journal
15206106 → ACNP
Volume
105
Issue
47
Year of publication
2001
Pages
11828 - 11833
Database
ISI
SICI code
1520-6106(20011129)105:47<11828:TIOCFO>2.0.ZU;2-Q
Abstract
We report here new results that further elucidate the role of buoyancy-driv en convective flows in determining the distribution of vapor mole fraction and temperature in the thermal diffusion cloud chamber. A two-dimensional m odel describing both diffusion and convection in the presence of chamber si dewalls is presented. The model equations are used to analyze 1-butanol and I-pentanol nucleation data obtained earlier. The results of the investigat ion show that convective flow is nearly always present and, in the cases co nsidered here, result in a reduction in the value of the calculated critica l supersaturation (as compared to the one-dimensional case). The dependence of critical supersaturation with total pressure reported earlier is smalle r but is not eliminated.