Expressions of the coupling constant for contradirectional two-wave mi
xing (CTWM) have been derived. The calculations show that the energy t
ransfer in CTWM has some unique characteristics different from the for
ward two-wave mixing (FTWM), in which the energy transfer direction is
dependent on the two beam orientations with respect to the crystal po
lar axis and the sign of the light-induced carriers as well as the ele
ctro-optic coefficients. As a result, the CTWM can have a reverse ener
gy transfer direction to the FTWM under a certain condition. The exper
imental results in two typical crystals of Rh-doped BaTiO3 and in Ce-d
oped strontium barium niobate (SBN:Ce) demonstrate the theoretical inv
estigations very well. (C) 1997 Elsevier Science B.V.