A neutron-scanning device was developed for measuring accurate neutron dens
ities of BWR high burn-up fuels up to 65 GWd tU(-1). Characteristic test of
this device was done with a Cf-252 source and adopted to measure axial dis
tributions of neutron densities of BWR spent fuels with various enrichments
(2.0-3.4%), which had been irradiated up to 60 GWd tU(-1) at Fukushima Dai
ni Nuclear Power Station Unit 2(2F-2). We found the measured neutron densit
ies were proportional to about fourth power of the corresponding burn-up va
lues. The neutron densities calculated by the ORIGEN2.1 code and various cr
oss section libraries showed good agreements with the measured ones in prof
ile and absolute value except for BWR-UE file mainly based on ENDF/B-IV. Th
e BS240J32 library based on JENDL3.2 was the best among the investigated li
braries. (C) 2001 Elsevier Science B.V. All rights reserved.