MAGNETIC QUENCHING EFFECTS ON LONG-LIVED POSITRONIUM STATES IN ZEOSIL

Citation
G. Duplatre et al., MAGNETIC QUENCHING EFFECTS ON LONG-LIVED POSITRONIUM STATES IN ZEOSIL, Journal of radioanalytical and nuclear chemistry, 211(1), 1996, pp. 225-235
Citations number
9
Categorie Soggetti
Chemistry Analytical","Nuclear Sciences & Tecnology","Chemistry Inorganic & Nuclear
ISSN journal
02365731
Volume
211
Issue
1
Year of publication
1996
Pages
225 - 235
Database
ISI
SICI code
0236-5731(1996)211:1<225:MQEOLP>2.0.ZU;2-4
Abstract
Positron annihilation data collected for zeosil (a zeolite-type solid allowing abundant Ps formation) are discussed, with particular attenti on payed to the longest-lived positronium states as observed in lifeti me spectroscopy experiments. To unravel the nature of these components , additional information was sought by applying an external magnetic f ield and by recording the total energy distribution of the annihilatio n radiation. From both the lifetime and the extended Doppler spectra, it is shown that positronium presents a very long-lived component with a relative intensity of ca. 30% and a lifetime close to the intrinsic tripler lifetime (140 ns), therefore undergoing almost no pick-off an nihilation. From the magnetic field experiments, the contact density p arameter has a value of essentially 1, which is characteristic of an u nperturbed triplet Ps state in vacuo. This positronium state therefore does not appear to interact with the medium.