G. Duplatre et al., MAGNETIC QUENCHING EFFECTS ON LONG-LIVED POSITRONIUM STATES IN ZEOSIL, Journal of radioanalytical and nuclear chemistry, 211(1), 1996, pp. 225-235
Positron annihilation data collected for zeosil (a zeolite-type solid
allowing abundant Ps formation) are discussed, with particular attenti
on payed to the longest-lived positronium states as observed in lifeti
me spectroscopy experiments. To unravel the nature of these components
, additional information was sought by applying an external magnetic f
ield and by recording the total energy distribution of the annihilatio
n radiation. From both the lifetime and the extended Doppler spectra,
it is shown that positronium presents a very long-lived component with
a relative intensity of ca. 30% and a lifetime close to the intrinsic
tripler lifetime (140 ns), therefore undergoing almost no pick-off an
nihilation. From the magnetic field experiments, the contact density p
arameter has a value of essentially 1, which is characteristic of an u
nperturbed triplet Ps state in vacuo. This positronium state therefore
does not appear to interact with the medium.