Previously, it has been recognized that radio halos in galaxy clusters are
preferentially associated with merging systems, as indicated by substructur
e in the X-ray images and temperature maps. Since, however, many clusters w
ithout radio halos also possess substructure, the role of mergers in the fo
rmation of radio halos has remained unclear. By using power ratios to relat
e gravitational potential fluctuations to substructure in X-ray images, we
provide the first quantitative comparison of the dynamical states of cluste
rs possessing radio halos. A correlation between the 1.4 GHz power (P-1.4)
of the radio halo (or relic) and the magnitude of the dipole power ratio (P
-1/P-0) is discovered such that approximately P-1.4 proportional to P-1/P-0
; i.e., the strongest radio halos appear only in those clusters currently e
xperiencing the largest departures from a virialized state. From the additi
onal consideration of a small number of highly disturbed clusters without r
adio halos detected at 1.4 GHz and recalling that radio halos are more comm
on in clusters with high X-ray luminosity (Giovannini, Tordi, & Feretti), w
e argue that radio halos form preferentially in massive (L-x greater than o
r similar to 0.5 x 10(45) ergs s(-1)) clusters experiencing violent mergers
(P-1/P-0 greater than or similar to 0.5 x 10(-4)) that have seriously disr
upted the cluster core. The association of radio halos with massive, large-
P-1/P-0, core-disrupted clusters can account for both the vital role of mer
gers in accelerating the relativistic particles responsible for the radio e
mission as well as the rare occurrence of radio halos in cluster samples.