The feasibility of a carbon dioxide desorption cooling process using an ope
n reactor was studied. Easy control of the cooling phase and a relatively i
nteresting energy storage capacity were demonstrated. Beyond the applicatio
n examined, this process raises the problem of developing an adsorbent mate
rial with a high energy storage capacity and high heat- and mass-transfer p
roperties. A method for defining the ideal activated carbon was developed f
rom the Dubinin approach. Implementation of PX21, a commercial activated ca
rbon with the closest to ideal characteristics for this application, was pe
rformed using a thermoplastic-expanded natural graphite combination. Dynami
c simulation, validated with experimental data, demonstrated the interest o
f this product and defined perspectives for improvement.