The space-charge-field harmonics in the refractive-index grating generated
in a bismuth silicate crystal to which a square-wave external electric fiel
d is applied were examined theoretically and experimentally at high interfe
rence-pattern contrasts. The model taking into account three spatial harmon
ics ensures good agreement with experimental data for the fundamental- and
second-harmonic gratings. By fitting the experimental data with theoretical
curves, the acceptor concentration and the product of the carrier mobility
and recombination time in the crystal were evaluated.