Cr-substituted Finemet-type nanocrystalline alloy (Fe63.5Cr10Si13.5B9Cu1Nb3
) has been studied by differential scanning calorimetry, x-ray diffraction,
Mossbauer spectroscopy, and magnetic measurements. The Curie temperature o
f the remaining amorphous phase decreases as the crystalline volume fractio
n increases, reaching values below room temperature. This feature makes the
alloy adequate for studying the magnetic decoupling of the (Fe,Si) nanocry
stals at moderated temperatures and, in particular, the superparamagnetic r
elaxation in broad temperature and crystalline fraction ranges. It was show
n that the anomalous dependence of the coercive field on the annealing temp
erature can be satisfactorily explained assuming a dipolar-type interaction
between the crystallites. (C) 2001 American Institute of Physics.