Fa. Akeredolu et al., THE FLUX OF ANTHROPOGENIC TRACE-METALS INTO THE ARCTIC FROM THE MIDLATITUDES IN 1979 80/, Atmospheric environment, 28(8), 1994, pp. 1557-1572
The flux of trace metals into the Arctic atmosphere between 0 and 3.5
km altitude for the period July 1979-June 1980 was determined using a
chemical transport modeling approach used previously for sulfur. The t
otal annual flux of antimony, arsenic, cadmium, lead, zinc and vanadiu
m into the Arctic from Eurasia was 4,285,47,2400,1350 and 474 tonnes,
respectively. This represents 3.4,6.0,4.2,3.0,3.1 and 1.7% of the sour
ce emissions, respectively. In contrast, the corresponding flux of sul
fur was 2.2 million tonnes or 6.7% of the total emissions. The followi
ng percentage contributions to the total flux, of all six metals, by t
he source regions were calculated: western Europe (7-34%), eastern Eur
ope (42-54%) and the Soviet Union (21-39%). The model also showed that
in addition to a late winter (February, March) maximum input to the A
rctic, a peak was also observed in October. This peak was shown to hav
e resulted from an unusual set of synoptic conditions, which produced
a strong northerly flow into the Arctic around 0-degrees longitude in
October 1979. Comparison of the model-predicted trace metal concentrat
ions with a set of limited observations at existing sampling stations
close to the Arctic Circle (namely Ny Alesund in Spitsbergen, Jergul,
Skrova and Jan Mayen) showed agreement within a factor of 2-3.